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In 1959, she received yet another nomination for her role in The Nun's Story (1959). Audrey reached the pinnacle of her career when she played Holly Golightly in the delightful film Breakfast at Tiffany's (1961) in 1961. For this she received another nomination. She scored commercial success again in the espionage caper Charade (1963).

One of Audrey's most radiant roles was in the fine production of My Fair Lady (1964) in 1964. Her co-star, Rex Harrison, once was asked to identify his favorite leading lady. Without hesitation, he replied, "Audrey Hepburn in 'My Fair Lady.'" After a couple of other movies, most notably Two for the Road (1967), she hit pay dirt and another nomination in 1967's Wait Until Dark (1967). By the end of the sixties, after her divorce from actor Mel Ferrer, Audrey decided to retire while she was on top.

Later she married Dr. Andrea Dotti. From time to time, she would appear on the silver screen. One film of note was Robin and Marian (1976), with Sean Connery in 1976.

In 1988, Audrey became a special ambassador to the United Nations UNICEF fund helping children in Latin America and Africa, a position she retained until 1993. She was named to People's magazine as one of the 50 most beautiful people in the world. Her last film was Always (1989) in 1989.

Audrey Hepburn died on January 20, 1993 in Tolochnaz, Switzerland, from colon cancer. She had made a total of 31 high quality movies. Her elegance and style will always be remembered in film history as evidenced by her being named in Empire magazine's "The Top 100 Movie Stars of All Time."